Atomic-scale visualization of inertial dynamics

AM Lindenberg; Jörgen Larsson; K Sokolowski-Tinten; KJ Gaffney; C Blome; Ola Synnergren; J Sheppard; C Caleman; AG MacPhee; D Weinstein; DP Lowney; TK Allison; T Matthews; RW Falcone; AL Cavalieri; DM Fritz; SH Lee; PH Bucksbaum; DA Reis; J Rudati; PH Fuoss; CC Kao; DP Siddons; R Pahl; J Als-Nielsen; S Duesterer; R Ischebeck; H Schlarb; H Schulte-Schrepping; T Tschentscher; J Schneider; D von der Linde; O Hignette; F Sette; HN Chapman; RW Lee; T N Hansen; S Techert; JS Wark; M Bergh; G Huldt; D van der Spoel; N Timneanu; J Hajdu; RA Akre; E Bong; P Krejcik; J Arthur; S Brennan; K Luening; JB Hastings

doi:10.1126/science.1107996

Atomic-scale visualization of inertial dynamics

AM Lindenberg, Jörgen Larsson, K Sokolowski-Tinten, KJ Gaffney, C Blome, Ola Synnergren, J Sheppard, C Caleman, AG MacPhee, D Weinstein, DP Lowney, TK Allison, T Matthews, RW Falcone, AL Cavalieri, DM Fritz, SH Lee, PH Bucksbaum, DA Reis, J RudatiPH Fuoss, CC Kao, DP Siddons, R Pahl, J Als-Nielsen, S Duesterer, R Ischebeck, H Schlarb, H Schulte-Schrepping, T Tschentscher, J Schneider, D von der Linde, O Hignette, F Sette, HN Chapman, RW Lee, T N Hansen, S Techert, JS Wark, M Bergh, G Huldt, D van der Spoel, N Timneanu, J Hajdu, RA Akre, E Bong, P Krejcik, J Arthur, S Brennan, K Luening, JB Hastings

Atomic Physics

Research output: Contribution to journal › Article › peer-review

Abstract

The motion of atoms on interatomic potential energy surfaces is fundamental to the dynamics of liquids and solids. An accelerator-based source of femtosecond x-ray pulses allowed us to follow directly atomic displacements on an optically modified energy landscape, leading eventually to the transition from crystalline solid to disordered liquid. We show that, to first order in time, the dynamics are inertial, and we place constraints on the shape and curvature of the transition-state potential energy surface. Our measurements point toward analogies between this nonequilibrium phase transition and the short-time dynamics intrinsic to equilibrium liquids.

Original language	English
Pages (from-to)	392-395
Journal	Science
Volume	308
Issue number	5720
DOIs	https://doi.org/10.1126/science.1107996
Publication status	Published - 2005

Subject classification (UKÄ)

Atom and Molecular Physics and Optics

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10.1126/science.1107996

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Lindenberg, AM., Larsson, J., Sokolowski-Tinten, K., Gaffney, KJ., Blome, C., Synnergren, O., Sheppard, J., Caleman, C., MacPhee, AG., Weinstein, D., Lowney, DP., Allison, TK., Matthews, T., Falcone, RW., Cavalieri, AL., Fritz, DM., Lee, SH., Bucksbaum, PH., Reis, DA., ... Hastings, JB. (2005). Atomic-scale visualization of inertial dynamics. Science, 308(5720), 392-395. https://doi.org/10.1126/science.1107996

@article{f3a04695844f4350988071e2852b784e,

title = "Atomic-scale visualization of inertial dynamics",

abstract = "The motion of atoms on interatomic potential energy surfaces is fundamental to the dynamics of liquids and solids. An accelerator-based source of femtosecond x-ray pulses allowed us to follow directly atomic displacements on an optically modified energy landscape, leading eventually to the transition from crystalline solid to disordered liquid. We show that, to first order in time, the dynamics are inertial, and we place constraints on the shape and curvature of the transition-state potential energy surface. Our measurements point toward analogies between this nonequilibrium phase transition and the short-time dynamics intrinsic to equilibrium liquids.",

author = "AM Lindenberg and J{\"o}rgen Larsson and K Sokolowski-Tinten and KJ Gaffney and C Blome and Ola Synnergren and J Sheppard and C Caleman and AG MacPhee and D Weinstein and DP Lowney and TK Allison and T Matthews and RW Falcone and AL Cavalieri and DM Fritz and SH Lee and PH Bucksbaum and DA Reis and J Rudati and PH Fuoss and CC Kao and DP Siddons and R Pahl and J Als-Nielsen and S Duesterer and R Ischebeck and H Schlarb and H Schulte-Schrepping and T Tschentscher and J Schneider and {von der Linde}, D and O Hignette and F Sette and HN Chapman and RW Lee and Hansen, {T N} and S Techert and JS Wark and M Bergh and G Huldt and {van der Spoel}, D and N Timneanu and J Hajdu and RA Akre and E Bong and P Krejcik and J Arthur and S Brennan and K Luening and JB Hastings",

year = "2005",

doi = "10.1126/science.1107996",

language = "English",

volume = "308",

pages = "392--395",

journal = "Science",

issn = "1095-9203",

publisher = "American Association for the Advancement of Science (AAAS)",

number = "5720",

}

Lindenberg, AM, Larsson, J, Sokolowski-Tinten, K, Gaffney, KJ, Blome, C, Synnergren, O, Sheppard, J, Caleman, C, MacPhee, AG, Weinstein, D, Lowney, DP, Allison, TK, Matthews, T, Falcone, RW, Cavalieri, AL, Fritz, DM, Lee, SH, Bucksbaum, PH, Reis, DA, Rudati, J, Fuoss, PH, Kao, CC, Siddons, DP, Pahl, R, Als-Nielsen, J, Duesterer, S, Ischebeck, R, Schlarb, H, Schulte-Schrepping, H, Tschentscher, T, Schneider, J, von der Linde, D, Hignette, O, Sette, F, Chapman, HN, Lee, RW, Hansen, TN, Techert, S, Wark, JS, Bergh, M, Huldt, G, van der Spoel, D, Timneanu, N, Hajdu, J, Akre, RA, Bong, E, Krejcik, P, Arthur, J, Brennan, S, Luening, K & Hastings, JB 2005, 'Atomic-scale visualization of inertial dynamics', Science, vol. 308, no. 5720, pp. 392-395. https://doi.org/10.1126/science.1107996

TY - JOUR

T1 - Atomic-scale visualization of inertial dynamics

AU - Lindenberg, AM

AU - Larsson, Jörgen

AU - Sokolowski-Tinten, K

AU - Gaffney, KJ

AU - Blome, C

AU - Synnergren, Ola

AU - Sheppard, J

AU - Caleman, C

AU - MacPhee, AG

AU - Weinstein, D

AU - Lowney, DP

AU - Allison, TK

AU - Matthews, T

AU - Falcone, RW

AU - Cavalieri, AL

AU - Fritz, DM

AU - Lee, SH

AU - Bucksbaum, PH

AU - Reis, DA

AU - Rudati, J

AU - Fuoss, PH

AU - Kao, CC

AU - Siddons, DP

AU - Pahl, R

AU - Als-Nielsen, J

AU - Duesterer, S

AU - Ischebeck, R

AU - Schlarb, H

AU - Schulte-Schrepping, H

AU - Tschentscher, T

AU - Schneider, J

AU - von der Linde, D

AU - Hignette, O

AU - Sette, F

AU - Chapman, HN

AU - Lee, RW

AU - Hansen, T N

AU - Techert, S

AU - Wark, JS

AU - Bergh, M

AU - Huldt, G

AU - van der Spoel, D

AU - Timneanu, N

AU - Hajdu, J

AU - Akre, RA

AU - Bong, E

AU - Krejcik, P

AU - Arthur, J

AU - Brennan, S

AU - Luening, K

AU - Hastings, JB

PY - 2005

Y1 - 2005

N2 - The motion of atoms on interatomic potential energy surfaces is fundamental to the dynamics of liquids and solids. An accelerator-based source of femtosecond x-ray pulses allowed us to follow directly atomic displacements on an optically modified energy landscape, leading eventually to the transition from crystalline solid to disordered liquid. We show that, to first order in time, the dynamics are inertial, and we place constraints on the shape and curvature of the transition-state potential energy surface. Our measurements point toward analogies between this nonequilibrium phase transition and the short-time dynamics intrinsic to equilibrium liquids.

AB - The motion of atoms on interatomic potential energy surfaces is fundamental to the dynamics of liquids and solids. An accelerator-based source of femtosecond x-ray pulses allowed us to follow directly atomic displacements on an optically modified energy landscape, leading eventually to the transition from crystalline solid to disordered liquid. We show that, to first order in time, the dynamics are inertial, and we place constraints on the shape and curvature of the transition-state potential energy surface. Our measurements point toward analogies between this nonequilibrium phase transition and the short-time dynamics intrinsic to equilibrium liquids.

U2 - 10.1126/science.1107996

DO - 10.1126/science.1107996

M3 - Article

SN - 1095-9203

VL - 308

SP - 392

EP - 395

JO - Science

JF - Science

IS - 5720

ER -

Atomic-scale visualization of inertial dynamics

Abstract

Subject classification (UKÄ)

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