Dual Bethe-Salpeter equation for the multiorbital lattice susceptibility within dynamical mean-field theory

Erik G.C.P. Van Loon, Hugo U.R. Strand

Research output: Contribution to journalArticlepeer-review

Abstract

Dynamical mean-field theory describes the impact of strong local correlation effects in many-electron systems. While the single-particle spectral function is directly obtained within the formalism, two-particle susceptibilities can also be obtained by solving the Bethe-Salpeter equation. The solution requires handling infinite matrices in Matsubara frequency space. This is commonly treated using a finite frequency cutoff, resulting in slow linear convergence. A decomposition of the two-particle response in local and nonlocal contributions enables a reformulation of the Bethe-Salpeter equation inspired by the dual boson formalism. The reformulation has a drastically improved cubic convergence with respect to the frequency cutoff, considerably facilitating the calculation of susceptibilities in multi-orbital systems. This improved convergence arises from the fact that local contributions can be measured in the impurity solver. The dual Bethe-Salpeter equation uses the fully reducible vertex which is free from vertex divergences. We benchmark the approach on several systems including the spin susceptibility of strontium ruthenate Sr2RuO4, a strongly correlated Hund's metal with three active orbitals.

Original languageEnglish
Article number155157
JournalPhysical Review B
Volume109
Issue number15
DOIs
Publication statusPublished - 2024 Apr

Subject classification (UKÄ)

  • Condensed Matter Physics (including Material Physics, Nano Physics)

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