Formate dehydrogenase-modified carbon paste electrodes for amperometric detection of formate

Florentina Munteanu, D Gligor, IC Popescu, Lo Gorton

Research output: Contribution to journalArticlepeer-review

Abstract

A simple and inexpensive amperometric biosensor for formate detection was obtained by immobilization of for-mate dehydrogenase (FDH) on graphite powder, modified with a new phenothiazine derivative (DDDP; 16H, 18H-dibenzo[c,l]-7,9-dithia-16,18-diazapentacene). Two different enzyme environments were used: FDH was adsorbed on DDDP-modified graphite powder in the presence of polyethylenimine (PEI) as well as in its absence. In both cases, when 10 mM NAD(+) were added in the supporting electrolyte (phosphate buffer, pH 7.0), the biosensor developed a response to formate, obeying Michaelis-Menten kinetics with a linear domain up to 3 mM formate. The biosensor sensitivity, calculated as the ratio 1(max)/K-M(aPP), was better in the second case (0.962 mA/M), but the best detection limit (3 AM) was observed in the first case.
Original languageEnglish
Pages (from-to)25-30
JournalRevue Roumaine de Chimie
Volume51
Issue number1
Publication statusPublished - 2006

Bibliographical note

The information about affiliations in this record was updated in December 2015.
The record was previously connected to the following departments: Analytical Chemistry (S/LTH) (011001004)

Subject classification (UKÄ)

  • Analytical Chemistry

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