Halide perovskite artificial solids as a new platform to simulate collective phenomena in doped Mott insulators

Alessandra Milloch, Umberto Filippi, Massimo Capone, Dmitry Baranov, Liberato Manna, Claudio Giannetti

Research output: Contribution to conferenceAbstract

Abstract

The development of Quantum Simulators, artificial platforms where the predictions of many-body theories of correlated quantum materials can be tested in a controllable and tunable way, is one of the main challenges of condensed matter physics. We introduce artificial lattices made of lead halide perovskite nanocubes as a new platform to simulate and investigate the physics of correlated quantum materials. The ultrafast optical injection of quantum-confined excitons plays a similar role to doping in real materials. We show that, at large photo-doping, the exciton gas undergoes an excitonic Mott transition, which can be mapped on the insulator-to-metal transition of the Hubbard model in a magnetic field. At lower photo-doping, the long-range interactions drive the formation of a collective superradiant state, in which the phases of the excitons generated in each single perovskite nanocube are coherently locked. Our results demonstrate that time-resolved experiments span a parameter region of the Hubbard model in which long-range and phase-coherent orders emerge out of a doped Mott insulating phase. This physics is relevant for a broad class of phenomena, such as superconductivity and charge-density waves in correlated materials whose properties are captured by doped Hubbard models.
Original languageEnglish
Publication statusPublished - 2023 Sept 4
EventCMD30 FisMat 2023: Joint Conference of the Italian and European Community of Condensed Matter Physics - Politecnico di Milano and the Università degli Studi di Milano, Milan, Italy
Duration: 2023 Sept 42023 Sept 8
https://eventi.cnism.it/cmd30-fismat

Conference

ConferenceCMD30 FisMat 2023
Abbreviated titleCMD30 FisMat 2023
Country/TerritoryItaly
CityMilan
Period2023/09/042023/09/08
Internet address

Subject classification (UKÄ)

  • Condensed Matter Physics

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