Influence of an atomic resonance on the coherent control of the photoionization process

E. V. Gryzlova; P. Carpeggiani; M. M. Popova; M. D. Kiselev; N. Douguet; M. Reduzzi; M. Negro; A. Comby; H. Ahmadi; V. Wanie; M. C. Castrovilli; A. Fischer; P. Eng-Johnsson; M. Meyer; K. Bartschat; S. M. Burkov; T. Csizmadia; M. Dumergue; Sergei Kühn; N. G. Harshitha; M. Fule; F. Aeenehvand; F. Stienkemeier; D. Iablonskyi; K. Ueda; P. Finetti; M. Zangrando; N. Mahne; K. L. Ishikawa; O. Plekan; K. C. Prince; E. Allaria; L. Giannessi; C. Callegari; A. N. Grum-Grzhimailo; G. Sansone

doi:10.1103/PhysRevResearch.4.033231

Influence of an atomic resonance on the coherent control of the photoionization process

E. V. Gryzlova, P. Carpeggiani, M. M. Popova, M. D. Kiselev, N. Douguet, M. Reduzzi, M. Negro, A. Comby, H. Ahmadi, V. Wanie, M. C. Castrovilli, A. Fischer, P. Eng-Johnsson, M. Meyer, K. Bartschat, S. M. Burkov, T. Csizmadia, M. Dumergue, Sergei Kühn, N. G. HarshithaM. Fule, F. Aeenehvand, F. Stienkemeier, D. Iablonskyi, K. Ueda, P. Finetti, M. Zangrando, N. Mahne, K. L. Ishikawa, O. Plekan, K. C. Prince, E. Allaria, L. Giannessi, C. Callegari, A. N. Grum-Grzhimailo, G. Sansone

Research output: Contribution to journal › Article › peer-review

Abstract

In coherent control schemes, pathways connecting an initial and a final state can be independently controlled by manipulating the complex amplitudes of their transition matrix elements. For paths characterized by the absorption of multiple photons, these quantities depend on the magnitude and phase between the intermediate steps, and are expected to be strongly affected by the presence of resonances. We investigate the coherent control of the photoemission process in neon using a phase-controlled two-color extreme ultraviolet pulse with frequency in proximity of an excited energy state. Using helium as a reference, we show that the presence of such a resonance in neon modifies the amplitude and phase of the asymmetric emission of photoelectrons. Theoretical simulations based on perturbation theory are in fair agreement with the experimental observations.

Original language	English
Article number	033231
Journal	Physical Review Research
Volume	4
Issue number	3
DOIs	https://doi.org/10.1103/PhysRevResearch.4.033231
Publication status	Published - 2022 Jul

Subject classification (UKÄ)

Atom and Molecular Physics and Optics

Access to Document

10.1103/PhysRevResearch.4.033231

Cite this

Gryzlova, E. V., Carpeggiani, P., Popova, M. M., Kiselev, M. D., Douguet, N., Reduzzi, M., Negro, M., Comby, A., Ahmadi, H., Wanie, V., Castrovilli, M. C., Fischer, A., Eng-Johnsson, P., Meyer, M., Bartschat, K., Burkov, S. M., Csizmadia, T., Dumergue, M., Kühn, S., ... Sansone, G. (2022). Influence of an atomic resonance on the coherent control of the photoionization process. Physical Review Research, 4(3), Article 033231. https://doi.org/10.1103/PhysRevResearch.4.033231

@article{ec3c24cb04614d8198a461bc573e53ca,

title = "Influence of an atomic resonance on the coherent control of the photoionization process",

abstract = "In coherent control schemes, pathways connecting an initial and a final state can be independently controlled by manipulating the complex amplitudes of their transition matrix elements. For paths characterized by the absorption of multiple photons, these quantities depend on the magnitude and phase between the intermediate steps, and are expected to be strongly affected by the presence of resonances. We investigate the coherent control of the photoemission process in neon using a phase-controlled two-color extreme ultraviolet pulse with frequency in proximity of an excited energy state. Using helium as a reference, we show that the presence of such a resonance in neon modifies the amplitude and phase of the asymmetric emission of photoelectrons. Theoretical simulations based on perturbation theory are in fair agreement with the experimental observations.",

author = "Gryzlova, {E. V.} and P. Carpeggiani and Popova, {M. M.} and Kiselev, {M. D.} and N. Douguet and M. Reduzzi and M. Negro and A. Comby and H. Ahmadi and V. Wanie and Castrovilli, {M. C.} and A. Fischer and P. Eng-Johnsson and M. Meyer and K. Bartschat and Burkov, {S. M.} and T. Csizmadia and M. Dumergue and Sergei K{\"u}hn and Harshitha, {N. G.} and M. Fule and F. Aeenehvand and F. Stienkemeier and D. Iablonskyi and K. Ueda and P. Finetti and M. Zangrando and N. Mahne and Ishikawa, {K. L.} and O. Plekan and Prince, {K. C.} and E. Allaria and L. Giannessi and C. Callegari and Grum-Grzhimailo, {A. N.} and G. Sansone",

year = "2022",

month = jul,

doi = "10.1103/PhysRevResearch.4.033231",

language = "English",

volume = "4",

journal = "Physical Review Research",

issn = "2643-1564",

publisher = "American Physical Society",

number = "3",

}

Gryzlova, EV, Carpeggiani, P, Popova, MM, Kiselev, MD, Douguet, N, Reduzzi, M, Negro, M, Comby, A, Ahmadi, H, Wanie, V, Castrovilli, MC, Fischer, A, Eng-Johnsson, P, Meyer, M, Bartschat, K, Burkov, SM, Csizmadia, T, Dumergue, M, Kühn, S, Harshitha, NG, Fule, M, Aeenehvand, F, Stienkemeier, F, Iablonskyi, D, Ueda, K, Finetti, P, Zangrando, M, Mahne, N, Ishikawa, KL, Plekan, O, Prince, KC, Allaria, E, Giannessi, L, Callegari, C, Grum-Grzhimailo, AN & Sansone, G 2022, 'Influence of an atomic resonance on the coherent control of the photoionization process', Physical Review Research, vol. 4, no. 3, 033231. https://doi.org/10.1103/PhysRevResearch.4.033231

TY - JOUR

T1 - Influence of an atomic resonance on the coherent control of the photoionization process

AU - Gryzlova, E. V.

AU - Carpeggiani, P.

AU - Popova, M. M.

AU - Kiselev, M. D.

AU - Douguet, N.

AU - Reduzzi, M.

AU - Negro, M.

AU - Comby, A.

AU - Ahmadi, H.

AU - Wanie, V.

AU - Castrovilli, M. C.

AU - Fischer, A.

AU - Eng-Johnsson, P.

AU - Meyer, M.

AU - Bartschat, K.

AU - Burkov, S. M.

AU - Csizmadia, T.

AU - Dumergue, M.

AU - Kühn, Sergei

AU - Harshitha, N. G.

AU - Fule, M.

AU - Aeenehvand, F.

AU - Stienkemeier, F.

AU - Iablonskyi, D.

AU - Ueda, K.

AU - Finetti, P.

AU - Zangrando, M.

AU - Mahne, N.

AU - Ishikawa, K. L.

AU - Plekan, O.

AU - Prince, K. C.

AU - Allaria, E.

AU - Giannessi, L.

AU - Callegari, C.

AU - Grum-Grzhimailo, A. N.

AU - Sansone, G.

PY - 2022/7

Y1 - 2022/7

N2 - In coherent control schemes, pathways connecting an initial and a final state can be independently controlled by manipulating the complex amplitudes of their transition matrix elements. For paths characterized by the absorption of multiple photons, these quantities depend on the magnitude and phase between the intermediate steps, and are expected to be strongly affected by the presence of resonances. We investigate the coherent control of the photoemission process in neon using a phase-controlled two-color extreme ultraviolet pulse with frequency in proximity of an excited energy state. Using helium as a reference, we show that the presence of such a resonance in neon modifies the amplitude and phase of the asymmetric emission of photoelectrons. Theoretical simulations based on perturbation theory are in fair agreement with the experimental observations.

AB - In coherent control schemes, pathways connecting an initial and a final state can be independently controlled by manipulating the complex amplitudes of their transition matrix elements. For paths characterized by the absorption of multiple photons, these quantities depend on the magnitude and phase between the intermediate steps, and are expected to be strongly affected by the presence of resonances. We investigate the coherent control of the photoemission process in neon using a phase-controlled two-color extreme ultraviolet pulse with frequency in proximity of an excited energy state. Using helium as a reference, we show that the presence of such a resonance in neon modifies the amplitude and phase of the asymmetric emission of photoelectrons. Theoretical simulations based on perturbation theory are in fair agreement with the experimental observations.

U2 - 10.1103/PhysRevResearch.4.033231

DO - 10.1103/PhysRevResearch.4.033231

M3 - Article

AN - SCOPUS:85139260003

SN - 2643-1564

VL - 4

JO - Physical Review Research

JF - Physical Review Research

IS - 3

M1 - 033231

ER -

Influence of an atomic resonance on the coherent control of the photoionization process

Abstract

Subject classification (UKÄ)

Access to Document

Fingerprint

Cite this