Modelling multiphase aerosol-cloud processing with the 3-D CTM COSMO-MUSCAT: application for cloud events during HCCT-2010

Roland Schrödner; Ralf Wolke; Andreas Tilgner; Dominik van Pinxteren; Hartmut Herrmann

doi:10.1007/978-3-319-57645-9_91

Modelling multiphase aerosol-cloud processing with the 3-D CTM COSMO-MUSCAT: application for cloud events during HCCT-2010

Roland Schrödner, Ralf Wolke, Andreas Tilgner, Dominik van Pinxteren, Hartmut Herrmann

Leibniz Institute for Tropospheric Research (TROPOS)

Research output: Chapter in Book/Report/Conference proceeding › Book chapter › Research › peer-review

Abstract

The online-coupled 3-D chemistry transport model COSMO-MUSCAT was enhanced by a detailed description of aqueous phase chemical processes. The aqueous phase chemistry is represented by the detailed chemical mechanism CAPRAM 3.0i reduced (C3.0RED). In addition, the deposition schemes were improved in order to account for the deposition of matter incorporated in cloud droplets of ground layer clouds and fogs. The extended model system was applied for real 3‑D case studies connected to the field experiment HCCT-2010 (Hill Cap Cloud Thuringia, 2010). Process and sensitivity studies were conducted and the results were compared to the available measurements during HCCT-2010. The studies indicate the requirement to consider chemical cloud effects in regional CTMs because of their key impacts on e.g., oxidation capacity in the gas and aqueous phase, formation of organic and inorganic particulate matter, and droplet acidity.

Original language	English
Title of host publication	Springer Proceedings in Complexity
Publisher	Springer
Pages	587-592
Number of pages	6
DOIs	https://doi.org/10.1007/978-3-319-57645-9_91
Publication status	Published - 2017

Subject classification (UKÄ)

Environmental Sciences
Meteorology and Atmospheric Sciences

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10.1007/978-3-319-57645-9_91

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title = "Modelling multiphase aerosol-cloud processing with the 3-D CTM COSMO-MUSCAT: application for cloud events during HCCT-2010",

abstract = "The online-coupled 3-D chemistry transport model COSMO-MUSCAT was enhanced by a detailed description of aqueous phase chemical processes. The aqueous phase chemistry is represented by the detailed chemical mechanism CAPRAM 3.0i reduced (C3.0RED). In addition, the deposition schemes were improved in order to account for the deposition of matter incorporated in cloud droplets of ground layer clouds and fogs. The extended model system was applied for real 3‑D case studies connected to the field experiment HCCT-2010 (Hill Cap Cloud Thuringia, 2010). Process and sensitivity studies were conducted and the results were compared to the available measurements during HCCT-2010. The studies indicate the requirement to consider chemical cloud effects in regional CTMs because of their key impacts on e.g., oxidation capacity in the gas and aqueous phase, formation of organic and inorganic particulate matter, and droplet acidity.",

author = "Roland Schr{\"o}dner and Ralf Wolke and Andreas Tilgner and {van Pinxteren}, Dominik and Hartmut Herrmann",

year = "2017",

doi = "10.1007/978-3-319-57645-9_91",

language = "English",

pages = "587--592",

booktitle = "Springer Proceedings in Complexity",

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T1 - Modelling multiphase aerosol-cloud processing with the 3-D CTM COSMO-MUSCAT

T2 - application for cloud events during HCCT-2010

AU - Schrödner, Roland

AU - Wolke, Ralf

AU - Tilgner, Andreas

AU - van Pinxteren, Dominik

AU - Herrmann, Hartmut

PY - 2017

Y1 - 2017

N2 - The online-coupled 3-D chemistry transport model COSMO-MUSCAT was enhanced by a detailed description of aqueous phase chemical processes. The aqueous phase chemistry is represented by the detailed chemical mechanism CAPRAM 3.0i reduced (C3.0RED). In addition, the deposition schemes were improved in order to account for the deposition of matter incorporated in cloud droplets of ground layer clouds and fogs. The extended model system was applied for real 3‑D case studies connected to the field experiment HCCT-2010 (Hill Cap Cloud Thuringia, 2010). Process and sensitivity studies were conducted and the results were compared to the available measurements during HCCT-2010. The studies indicate the requirement to consider chemical cloud effects in regional CTMs because of their key impacts on e.g., oxidation capacity in the gas and aqueous phase, formation of organic and inorganic particulate matter, and droplet acidity.

AB - The online-coupled 3-D chemistry transport model COSMO-MUSCAT was enhanced by a detailed description of aqueous phase chemical processes. The aqueous phase chemistry is represented by the detailed chemical mechanism CAPRAM 3.0i reduced (C3.0RED). In addition, the deposition schemes were improved in order to account for the deposition of matter incorporated in cloud droplets of ground layer clouds and fogs. The extended model system was applied for real 3‑D case studies connected to the field experiment HCCT-2010 (Hill Cap Cloud Thuringia, 2010). Process and sensitivity studies were conducted and the results were compared to the available measurements during HCCT-2010. The studies indicate the requirement to consider chemical cloud effects in regional CTMs because of their key impacts on e.g., oxidation capacity in the gas and aqueous phase, formation of organic and inorganic particulate matter, and droplet acidity.

U2 - 10.1007/978-3-319-57645-9_91

DO - 10.1007/978-3-319-57645-9_91

M3 - Book chapter

AN - SCOPUS:85060480203

SP - 587

EP - 592

BT - Springer Proceedings in Complexity

PB - Springer

ER -

Modelling multiphase aerosol-cloud processing with the 3-D CTM COSMO-MUSCAT: application for cloud events during HCCT-2010

Abstract

Subject classification (UKÄ)

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