TY - JOUR
T1 - Mollow-like Triplets in Ultrafast Resonant Absorption
AU - Stenquist, Axel
AU - Zapata, Felipe
AU - Olofsson, Edvin
AU - Liao, Yijie
AU - Svegborn, Elna
AU - Bruhnke, Jakob Nicolai
AU - Verdozzi, Claudio
AU - Dahlström, Jan Marcus
PY - 2024/8
Y1 - 2024/8
N2 - We show that resonant absorption of smooth laser fields can yield Mollow-like triplet patterns. General conditions for such triplets are derived and illustrated with a super-Gaussian pulse sequence. Gaussian pulses cannot exhibit triplets, super-Gaussian pulses can form triplets depending on the pulse area, and flattop pulses can produce absorption triplets after one Rabi cycle. Our results are compared side by side with resonance fluorescence to emphasize similarities and differences between these unlike observables. In the high-intensity limit, we show that the central absorption peak is asymmetric, which we attribute to nonlinear photoionization, beyond two-level atomic physics.
AB - We show that resonant absorption of smooth laser fields can yield Mollow-like triplet patterns. General conditions for such triplets are derived and illustrated with a super-Gaussian pulse sequence. Gaussian pulses cannot exhibit triplets, super-Gaussian pulses can form triplets depending on the pulse area, and flattop pulses can produce absorption triplets after one Rabi cycle. Our results are compared side by side with resonance fluorescence to emphasize similarities and differences between these unlike observables. In the high-intensity limit, we show that the central absorption peak is asymmetric, which we attribute to nonlinear photoionization, beyond two-level atomic physics.
U2 - 10.1103/PhysRevLett.133.063202
DO - 10.1103/PhysRevLett.133.063202
M3 - Article
C2 - 39178456
AN - SCOPUS:85201303125
SN - 0031-9007
VL - 133
JO - Physical Review Letters
JF - Physical Review Letters
IS - 6
M1 - 063202
ER -