Abstract
The nuclear dynamics in the Nt 1s→π* in nitrous oxide was studied using the high resolution resonant Auger spectroscopy and ab initio quantum chemical calculations. For probing the nuclear motion of the system in the core-excited state, the frequency detuning technique was used. The results showed changes in vibrational structure for the Auger decay spectra and a strong influence of nuclear motion on the electronic decay.
Original language | English |
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Pages (from-to) | 864-869 |
Number of pages | 6 |
Journal | Journal of Chemical Physics |
Volume | 115 |
Issue number | 2 |
DOIs | |
Publication status | Published - 2001 Jul 8 |