Plasmon single- and multi-quantum excitation in free metal clusters as seen by photoelectron spectroscopy.

Tomas Andersson, Chaofan Zhang, Aldana Rosso, I Bradeanu, Sébastien Legendre, Sophie Canton, Maxim Tchaplyguine, Gunnar Öhrwall, Stacey Ristinmaa Sörensen, S Svensson, Nils Mårtensson, O Björneholm

Research output: Contribution to journalArticlepeer-review

10 Citations (SciVal)

Abstract

Plasmons are investigated in free nanoscale Na, Mg, and K metal clusters using synchrotron radiation-based x-ray photoelectron spectroscopy. The core levels for which the response from bulk and surface atoms can be resolved are probed over an extended binding energy range to include the plasmon loss features. In all species the features due to fundamental plasmons are identified, and in Na and K also those due to either the first order plasmon overtones or sequential plasmon excitation are observed. These features are discussed in view of earlier results for planar macroscopic samples and free clusters of the same materials.
Original languageEnglish
Article number094511
JournalJournal of Chemical Physics
Volume134
Issue number9
DOIs
Publication statusPublished - 2011

Bibliographical note

The information about affiliations in this record was updated in December 2015.
The record was previously connected to the following departments: Max-laboratory (011012005), Chemical Physics (S) (011001060), Synchrotron Radiation Research (011013009)

Subject classification (UKÄ)

  • Atom and Molecular Physics and Optics

Fingerprint

Dive into the research topics of 'Plasmon single- and multi-quantum excitation in free metal clusters as seen by photoelectron spectroscopy.'. Together they form a unique fingerprint.

Cite this