Rydberg-Resolved Resonant Inelastic Soft X-Ray Scattering: Dynamics at Core Ionization Thresholds

J. -E. Rubensson; J. Söderström; C. Binggeli; J. Gråsjö; J. Andersson; Conny Såthe; Franz Hennies; V. Bisogni; Y. Huang; P. Olalde; T. Schmitt; V. N. Strocov; A. Föhlisch; B. Kennedy; A. Pietzsch

doi:10.1103/PhysRevLett.114.133001

Rydberg-Resolved Resonant Inelastic Soft X-Ray Scattering: Dynamics at Core Ionization Thresholds

J. -E. Rubensson, J. Söderström, C. Binggeli, J. Gråsjö, J. Andersson, Conny Såthe, Franz Hennies, V. Bisogni, Y. Huang, P. Olalde, T. Schmitt, V. N. Strocov, A. Föhlisch, B. Kennedy, A. Pietzsch

MAX IV Laboratory

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Abstract

Resonant inelastic x-ray scattering spectra excited in the immediate vicinity of the core-level ionization thresholds of N-2 have been recorded. Final states of well-resolved symmetry-selected Rydberg series converging to valence-level ionization thresholds with vibrational excitations are observed. The results are well described by a quasi-two-step model which assumes that the excited electron is unaffected by the radiative decay. This threshold dynamics simplifies the interpretation of resonant inelastic x-ray scattering spectra considerably and facilitates characterization of low-energy excited final states in molecular systems.

Original language	English
Article number	133001
Journal	Physical Review Letters
Volume	114
Issue number	13
DOIs	https://doi.org/10.1103/PhysRevLett.114.133001
Publication status	Published - 2015

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Physical Sciences

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10.1103/PhysRevLett.114.133001

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Rubensson, J. -E., Söderström, J., Binggeli, C., Gråsjö, J., Andersson, J., Såthe, C., Hennies, F., Bisogni, V., Huang, Y., Olalde, P., Schmitt, T., Strocov, V. N., Föhlisch, A., Kennedy, B., & Pietzsch, A. (2015). Rydberg-Resolved Resonant Inelastic Soft X-Ray Scattering: Dynamics at Core Ionization Thresholds. Physical Review Letters, 114(13), [133001]. https://doi.org/10.1103/PhysRevLett.114.133001

Rubensson, J. -E. ; Söderström, J. ; Binggeli, C. ; Gråsjö, J. ; Andersson, J. ; Såthe, Conny ; Hennies, Franz ; Bisogni, V. ; Huang, Y. ; Olalde, P. ; Schmitt, T. ; Strocov, V. N. ; Föhlisch, A. ; Kennedy, B. ; Pietzsch, A. / Rydberg-Resolved Resonant Inelastic Soft X-Ray Scattering: Dynamics at Core Ionization Thresholds. In: Physical Review Letters. 2015 ; Vol. 114, No. 13.

@article{4eef5fcc9a214df0af7d5688dcb80386,

title = "Rydberg-Resolved Resonant Inelastic Soft X-Ray Scattering: Dynamics at Core Ionization Thresholds",

abstract = "Resonant inelastic x-ray scattering spectra excited in the immediate vicinity of the core-level ionization thresholds of N-2 have been recorded. Final states of well-resolved symmetry-selected Rydberg series converging to valence-level ionization thresholds with vibrational excitations are observed. The results are well described by a quasi-two-step model which assumes that the excited electron is unaffected by the radiative decay. This threshold dynamics simplifies the interpretation of resonant inelastic x-ray scattering spectra considerably and facilitates characterization of low-energy excited final states in molecular systems.",

author = "Rubensson, {J. -E.} and J. S{\"o}derstr{\"o}m and C. Binggeli and J. Gr{\aa}sj{\"o} and J. Andersson and Conny S{\aa}the and Franz Hennies and V. Bisogni and Y. Huang and P. Olalde and T. Schmitt and Strocov, {V. N.} and A. F{\"o}hlisch and B. Kennedy and A. Pietzsch",

year = "2015",

doi = "10.1103/PhysRevLett.114.133001",

language = "English",

volume = "114",

journal = "Physical Review Letters",

issn = "1079-7114",

publisher = "American Physical Society",

number = "13",

}

Rubensson, J-E, Söderström, J, Binggeli, C, Gråsjö, J, Andersson, J, Såthe, C , Hennies, F, Bisogni, V, Huang, Y, Olalde, P, Schmitt, T, Strocov, VN, Föhlisch, A, Kennedy, B & Pietzsch, A 2015, 'Rydberg-Resolved Resonant Inelastic Soft X-Ray Scattering: Dynamics at Core Ionization Thresholds', Physical Review Letters, vol. 114, no. 13, 133001. https://doi.org/10.1103/PhysRevLett.114.133001

Rydberg-Resolved Resonant Inelastic Soft X-Ray Scattering: Dynamics at Core Ionization Thresholds. / Rubensson, J. -E.; Söderström, J.; Binggeli, C.; Gråsjö, J.; Andersson, J.; Såthe, Conny ; Hennies, Franz; Bisogni, V.; Huang, Y.; Olalde, P.; Schmitt, T.; Strocov, V. N.; Föhlisch, A.; Kennedy, B.; Pietzsch, A.

In: Physical Review Letters, Vol. 114, No. 13, 133001, 2015.

Research output: Contribution to journal › Article › peer-review

TY - JOUR

T1 - Rydberg-Resolved Resonant Inelastic Soft X-Ray Scattering: Dynamics at Core Ionization Thresholds

AU - Rubensson, J. -E.

AU - Söderström, J.

AU - Binggeli, C.

AU - Gråsjö, J.

AU - Andersson, J.

AU - Såthe, Conny

AU - Hennies, Franz

AU - Bisogni, V.

AU - Huang, Y.

AU - Olalde, P.

AU - Schmitt, T.

AU - Strocov, V. N.

AU - Föhlisch, A.

AU - Kennedy, B.

AU - Pietzsch, A.

PY - 2015

Y1 - 2015

N2 - Resonant inelastic x-ray scattering spectra excited in the immediate vicinity of the core-level ionization thresholds of N-2 have been recorded. Final states of well-resolved symmetry-selected Rydberg series converging to valence-level ionization thresholds with vibrational excitations are observed. The results are well described by a quasi-two-step model which assumes that the excited electron is unaffected by the radiative decay. This threshold dynamics simplifies the interpretation of resonant inelastic x-ray scattering spectra considerably and facilitates characterization of low-energy excited final states in molecular systems.

AB - Resonant inelastic x-ray scattering spectra excited in the immediate vicinity of the core-level ionization thresholds of N-2 have been recorded. Final states of well-resolved symmetry-selected Rydberg series converging to valence-level ionization thresholds with vibrational excitations are observed. The results are well described by a quasi-two-step model which assumes that the excited electron is unaffected by the radiative decay. This threshold dynamics simplifies the interpretation of resonant inelastic x-ray scattering spectra considerably and facilitates characterization of low-energy excited final states in molecular systems.

U2 - 10.1103/PhysRevLett.114.133001

DO - 10.1103/PhysRevLett.114.133001

M3 - Article

C2 - 25884123

VL - 114

JO - Physical Review Letters

JF - Physical Review Letters

SN - 1079-7114

IS - 13

M1 - 133001

ER -

Rydberg-Resolved Resonant Inelastic Soft X-Ray Scattering: Dynamics at Core Ionization Thresholds

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