Simultaneous temporally and spectrally resolved Raman coherences with single-shot fs/ns rotational CARS

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Abstract

A novel technique for studies of the dynamics of molecular coherences has been developed. The concept is based on prompt excitation using broadband femtosecond (fs) laser pulses, whereupon a narrowband nanosecond (ns) laser pulse probes the fast dynamics of the coherences. Detection of the spectrally dispersed coherent signal using a streak camera allows simultaneous spectrally and temporally resolved studies of all excited coherences in a single-shot acquisition. Here we demonstrate the high capacity and versatility of this hybrid fs/ns coherent anti-Stokes Raman scattering (CARS) technique through some illustrative examples, all single-shot measurements, namely time-resolved studies of rotational Raman coherences in nitrogen and air, dynamics of Stark effect on rotational lines, and beating phenomena originating from close-lying rotational lines.

Original languageEnglish
Pages (from-to)308-311
Number of pages4
JournalOptics Letters
Volume45
Issue number2
DOIs
Publication statusPublished - 2020

Subject classification (UKÄ)

  • Atom and Molecular Physics and Optics

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