Size determination of free metal clusters by core-level photoemission from different initial charge states

Sergey Peredkov; Stacey Ristinmaa Sörensen; Aldana Rosso; G. Ohrwall; M. Lundwall; T. Rander; A. Lindblad; H. Bergersen; W. Pokapanich; S. Svensson; O. Bjorneholm; Nils Mårtensson; Maxim Tchaplyguine

doi:10.1103/PhysRevB.76.081402

Size determination of free metal clusters by core-level photoemission from different initial charge states

Sergey Peredkov, Stacey Ristinmaa Sörensen, Aldana Rosso, G. Ohrwall, M. Lundwall, T. Rander, A. Lindblad, H. Bergersen, W. Pokapanich, S. Svensson, O. Bjorneholm, Nils Mårtensson, Maxim Tchaplyguine

Uppsala University

Research output: Contribution to journal › Article › peer-review

Abstract

We present the study of free nanoscale lead clusters using photoelectron spectroscopy and synchrotron radiation. Pb 5d core-level spectra reveal the presence of different initial charge states of the clusters created by the magnetron-based source. We suggest a method for determining the cluster size from the charge-dependent core level binding energies. Both the core-level and the valence spectra demonstrate that we have created free metallic clusters with essentially the same electronic structure as the solid.

Original language	English
Article number	081402(R)
Journal	Physical Review B (Condensed Matter and Materials Physics)
Volume	76
Issue number	8
DOIs	https://doi.org/10.1103/PhysRevB.76.081402
Publication status	Published - 2007

Subject classification (UKÄ)

Atom and Molecular Physics and Optics
Physical Sciences
Natural Sciences

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10.1103/PhysRevB.76.081402

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Peredkov, S., Ristinmaa Sörensen, S., Rosso, A., Ohrwall, G., Lundwall, M., Rander, T., Lindblad, A., Bergersen, H., Pokapanich, W., Svensson, S., Bjorneholm, O., Mårtensson, N., & Tchaplyguine, M. (2007). Size determination of free metal clusters by core-level photoemission from different initial charge states. Physical Review B (Condensed Matter and Materials Physics), 76(8), Article 081402(R). https://doi.org/10.1103/PhysRevB.76.081402

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title = "Size determination of free metal clusters by core-level photoemission from different initial charge states",

abstract = "We present the study of free nanoscale lead clusters using photoelectron spectroscopy and synchrotron radiation. Pb 5d core-level spectra reveal the presence of different initial charge states of the clusters created by the magnetron-based source. We suggest a method for determining the cluster size from the charge-dependent core level binding energies. Both the core-level and the valence spectra demonstrate that we have created free metallic clusters with essentially the same electronic structure as the solid.",

author = "Sergey Peredkov and {Ristinmaa S{\"o}rensen}, Stacey and Aldana Rosso and G. Ohrwall and M. Lundwall and T. Rander and A. Lindblad and H. Bergersen and W. Pokapanich and S. Svensson and O. Bjorneholm and Nils M{\aa}rtensson and Maxim Tchaplyguine",

year = "2007",

doi = "10.1103/PhysRevB.76.081402",

language = "English",

volume = "76",

journal = "Physical Review B (Condensed Matter and Materials Physics)",

issn = "1098-0121",

publisher = "American Physical Society",

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Peredkov, S, Ristinmaa Sörensen, S , Rosso, A, Ohrwall, G, Lundwall, M, Rander, T, Lindblad, A, Bergersen, H, Pokapanich, W, Svensson, S, Bjorneholm, O, Mårtensson, N & Tchaplyguine, M 2007, 'Size determination of free metal clusters by core-level photoemission from different initial charge states', Physical Review B (Condensed Matter and Materials Physics), vol. 76, no. 8, 081402(R). https://doi.org/10.1103/PhysRevB.76.081402

TY - JOUR

T1 - Size determination of free metal clusters by core-level photoemission from different initial charge states

AU - Peredkov, Sergey

AU - Ristinmaa Sörensen, Stacey

AU - Rosso, Aldana

AU - Ohrwall, G.

AU - Lundwall, M.

AU - Rander, T.

AU - Lindblad, A.

AU - Bergersen, H.

AU - Pokapanich, W.

AU - Svensson, S.

AU - Bjorneholm, O.

AU - Mårtensson, Nils

AU - Tchaplyguine, Maxim

PY - 2007

Y1 - 2007

N2 - We present the study of free nanoscale lead clusters using photoelectron spectroscopy and synchrotron radiation. Pb 5d core-level spectra reveal the presence of different initial charge states of the clusters created by the magnetron-based source. We suggest a method for determining the cluster size from the charge-dependent core level binding energies. Both the core-level and the valence spectra demonstrate that we have created free metallic clusters with essentially the same electronic structure as the solid.

AB - We present the study of free nanoscale lead clusters using photoelectron spectroscopy and synchrotron radiation. Pb 5d core-level spectra reveal the presence of different initial charge states of the clusters created by the magnetron-based source. We suggest a method for determining the cluster size from the charge-dependent core level binding energies. Both the core-level and the valence spectra demonstrate that we have created free metallic clusters with essentially the same electronic structure as the solid.

U2 - 10.1103/PhysRevB.76.081402

DO - 10.1103/PhysRevB.76.081402

M3 - Article

SN - 1098-0121

VL - 76

JO - Physical Review B (Condensed Matter and Materials Physics)

JF - Physical Review B (Condensed Matter and Materials Physics)

IS - 8

M1 - 081402(R)

ER -

Size determination of free metal clusters by core-level photoemission from different initial charge states

Abstract

Subject classification (UKÄ)

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