Nuclear and electronic dynamics in atoms and molecules are the foundation of many physical processes and chemical reactions. Often, these dynamics take place on timescales so much shorter than those commonly encountered that they are called ultrafast.
In order to study ultrafast phenomena, time-resolved techniques such as pump-probe experiments, involving ultrafast light pulses, are necessary. For these experiments to be successful, the properties of ultrafast light pulses must be carefully controlled and examined in order to discern their influence on the experiment.
This thesis deals with the spatial and temporal properties of XUV light, generated through the process of high-order harmonic generation in gases, using an intense IR laser beam. The influence of the spatial properties of this generating laser on the XUV has been studied, as has the influence of the XUV light's spatial properties on its focusability and peak intensity.
The generated high-order harmonics are also used to study physical phenomena such as multiphoton ionization, something that requires high intensities. An instrument for simultaneous studies of ions and electrons produced by photoionization is also presented.
The efforts towards ultrafast pump-probe experiments include designs for interferometer setups to enable these experiments. Some preliminary results of interferometer testing are also given, including a proof of principle of XUV-IR pump-probe experiments on the Lund Laser Centre intense XUV beamline.
|Translated title of the contribution
|Spatiella och tidsmässiga aspekter av intensiva attosekundpulser för pump-prob-experiment
- Eng-Johnsson, Per, Supervisor
- L'Huillier, Anne, Assistant supervisor
|2019 May 17
|Place of Publication
|Published - 2019 Apr 23
Place: Rydbergsalen, Fysicum, Professorsgatan 1, Lund University, Faculty of Engineering LTH
Name: Mével, Eric
Affiliation: Université de Bordeaux, France
- Atom and Molecular Physics and Optics
- Other Engineering and Technologies not elsewhere specified
- ultrafast lasers
- ultrafast optics
- attosecond pulses
- pump-probe experiments
- XUV light
- XUV focusing
- wavefront sensing
- XUV optics
- X-ray optics
- Fysicumarkivet A:2019:Wikmark