Spatial quantum beats in vibrational resonant inelastic soft x-ray scattering at dissociating States in oxygen.

Annette Pietzsch; Y Sun; Franz Hennies; Z Rinkevicius; H O Karlsson; T Schmitt; V N Strocov; J Andersson; B Kennedy; J Schlappa; A Föhlisch; J-E Rubensson; F Gel'mukhanov

doi:10.1103/PhysRevLett.106.153004

Spatial quantum beats in vibrational resonant inelastic soft x-ray scattering at dissociating States in oxygen.

Annette Pietzsch, Y Sun, Franz Hennies, Z Rinkevicius, H O Karlsson, T Schmitt, V N Strocov, J Andersson, B Kennedy, J Schlappa, A Föhlisch, J-E Rubensson, F Gel'mukhanov

MAX IV Laboratory

Research output: Contribution to journal › Article › peer-review

Abstract

Resonant inelastic soft x-ray scattering (RIXS) spectra excited at the 1σ_{g}→3σ_{u} resonance in gas-phase O_{2} show excitations due to the nuclear degrees of freedom with up to 35 well-resolved discrete vibronic states and a continuum due to the kinetic energy distribution of the separated atoms. The RIXS profile demonstrates spatial quantum beats caused by two interfering wave packets with different momenta as the atoms separate. Thomson scattering strongly affects both the spectral profile and the scattering anisotropy.

Original language	English
Article number	153004
Journal	Physical Review Letters
Volume	106
Issue number	15
DOIs	https://doi.org/10.1103/PhysRevLett.106.153004
Publication status	Published - 2011

Subject classification (UKÄ)

Natural Sciences
Physical Sciences

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10.1103/PhysRevLett.106.153004

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Pietzsch, A., Sun, Y., Hennies, F., Rinkevicius, Z., Karlsson, H. O., Schmitt, T., Strocov, V. N., Andersson, J., Kennedy, B., Schlappa, J., Föhlisch, A., Rubensson, J.-E., & Gel'mukhanov, F. (2011). Spatial quantum beats in vibrational resonant inelastic soft x-ray scattering at dissociating States in oxygen. Physical Review Letters, 106(15), Article 153004. https://doi.org/10.1103/PhysRevLett.106.153004

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title = "Spatial quantum beats in vibrational resonant inelastic soft x-ray scattering at dissociating States in oxygen.",

abstract = "Resonant inelastic soft x-ray scattering (RIXS) spectra excited at the 1σ\_\{g\}→3σ\_\{u\} resonance in gas-phase O\_\{2\} show excitations due to the nuclear degrees of freedom with up to 35 well-resolved discrete vibronic states and a continuum due to the kinetic energy distribution of the separated atoms. The RIXS profile demonstrates spatial quantum beats caused by two interfering wave packets with different momenta as the atoms separate. Thomson scattering strongly affects both the spectral profile and the scattering anisotropy.",

author = "Annette Pietzsch and Y Sun and Franz Hennies and Z Rinkevicius and Karlsson, \{H O\} and T Schmitt and Strocov, \{V N\} and J Andersson and B Kennedy and J Schlappa and A F{\"o}hlisch and J-E Rubensson and F Gel'mukhanov",

year = "2011",

doi = "10.1103/PhysRevLett.106.153004",

language = "English",

volume = "106",

journal = "Physical Review Letters",

issn = "1079-7114",

publisher = "American Physical Society",

number = "15",

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Pietzsch, A, Sun, Y, Hennies, F, Rinkevicius, Z, Karlsson, HO, Schmitt, T, Strocov, VN, Andersson, J, Kennedy, B, Schlappa, J, Föhlisch, A, Rubensson, J-E & Gel'mukhanov, F 2011, 'Spatial quantum beats in vibrational resonant inelastic soft x-ray scattering at dissociating States in oxygen.', Physical Review Letters, vol. 106, no. 15, 153004. https://doi.org/10.1103/PhysRevLett.106.153004

TY - JOUR

T1 - Spatial quantum beats in vibrational resonant inelastic soft x-ray scattering at dissociating States in oxygen.

AU - Pietzsch, Annette

AU - Sun, Y

AU - Hennies, Franz

AU - Rinkevicius, Z

AU - Karlsson, H O

AU - Schmitt, T

AU - Strocov, V N

AU - Andersson, J

AU - Kennedy, B

AU - Schlappa, J

AU - Föhlisch, A

AU - Rubensson, J-E

AU - Gel'mukhanov, F

PY - 2011

Y1 - 2011

N2 - Resonant inelastic soft x-ray scattering (RIXS) spectra excited at the 1σ_{g}→3σ_{u} resonance in gas-phase O_{2} show excitations due to the nuclear degrees of freedom with up to 35 well-resolved discrete vibronic states and a continuum due to the kinetic energy distribution of the separated atoms. The RIXS profile demonstrates spatial quantum beats caused by two interfering wave packets with different momenta as the atoms separate. Thomson scattering strongly affects both the spectral profile and the scattering anisotropy.

AB - Resonant inelastic soft x-ray scattering (RIXS) spectra excited at the 1σ_{g}→3σ_{u} resonance in gas-phase O_{2} show excitations due to the nuclear degrees of freedom with up to 35 well-resolved discrete vibronic states and a continuum due to the kinetic energy distribution of the separated atoms. The RIXS profile demonstrates spatial quantum beats caused by two interfering wave packets with different momenta as the atoms separate. Thomson scattering strongly affects both the spectral profile and the scattering anisotropy.

UR - https://www.scopus.com/pages/publications/79960623604

U2 - 10.1103/PhysRevLett.106.153004

DO - 10.1103/PhysRevLett.106.153004

M3 - Article

C2 - 21568552

SN - 1079-7114

VL - 106

JO - Physical Review Letters

JF - Physical Review Letters

IS - 15

M1 - 153004

ER -

Spatial quantum beats in vibrational resonant inelastic soft x-ray scattering at dissociating States in oxygen.

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