Unexpected Sensitivity of Nitrogen Ions Superradiant Emission on Pump Laser Wavelength and Duration

Yi Liu, Pengji Ding, Neven Ibrakovic, Samuel Bengtsson, Shihua Chen, Rostyslav Danylo, Emma R. Simpson, Esben W. Larsen, Xiang Zhang, Zhengquan Fan, Aurélien Houard, Johan Mauritsson, Anne L'Huillier, Cord L. Arnold, Songlin Zhuang, Vladimir Tikhonchuk, André Mysyrowicz

Research output: Contribution to journalArticlepeer-review

Abstract

Nitrogen molecules in ambient air exposed to an intense near-infrared femtosecond laser pulse give rise to cavity-free superradiant emission at 391.4 and 427.8 nm. An unexpected pulse duration-dependent cyclic variation of the superradiance intensity is observed when the central wavelength of the femtosecond pump laser pulse is finely tuned between 780 and 820 nm, and no signal occurs at the resonant wavelength of 782.8 nm (2ω782.8 nm=ω391.4 nm). On the basis of a semiclassical recollision model, we show that an interference of dipolar moments of excited ions created by electron recollisions explains this behavior.

Original languageEnglish
Article number203205
JournalPhysical Review Letters
Volume119
Issue number20
DOIs
Publication statusPublished - 2017 Nov 17

Subject classification (UKÄ)

  • Atom and Molecular Physics and Optics

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