Photoionization in the time and frequency domain

Research output: Contribution to journalArticle

Abstract

Ultrafast processes in matter, such as the electron emission following light absorption, can now be studied using ultrashort light pulses of attosecond duration (10−18 s) in the extreme ultraviolet spectral range. The lack of spectral resolution due to the use of short light pulses has raised issues in the interpretation of the experimental results and the comparison with theoretical calculations. We determine photoionization time delays in neon atoms over a 40 eV energy range with an interferometric technique combining high temporal and spectral resolution. We spectrally disentangle direct ionization from ionization with shake-up, in which a second electron is left in an excited state, and obtain excellent agreement with theoretical calculations, thereby solving a puzzle raised by 7-year-old measurements.

Details

Authors
Organisations
External organisations
  • University of Gothenburg
  • Stockholm University
Research areas and keywords

Subject classification (UKÄ) – MANDATORY

  • Atom and Molecular Physics and Optics
Original languageEnglish
Pages (from-to)893-896
JournalScience
Volume358
Issue number6365
Early online date2017 Nov 2
Publication statusPublished - 2017 Nov 17
Publication categoryResearch
Peer-reviewedYes