Plutonium remobilization in a humic-rich lake

Research output: Contribution to journalArticle

Abstract

Fresh water from Lake Svartsjon, Sweden, was collected and four fractions were prepared: (1) adsorption on DEAE, (2) flocculation with Ca2+, (3) co-precipitation with Fe hydrous oxide and (4) co-precipitation with Mn hydrous oxide. The plutonium level in the lake is 65 fg/l (222 mu Bq/l), measured by ICP-QMS and ICP-SFMS. Pronounced accumulation in fractions (1) (34%) and (2) (66%), combined with observed levels of organic matter indicate that plutonium is predominantly associated with organic matter. Measurements of isotopic ratios indicate that 77% of the plutonium originates from weapons testing and the remaining appears to originate from the Chernobyl accident.

Details

Authors
  • C. Greis
  • A. Duker
  • B. Allard
  • Per Roos
  • Elis Holm
Organisations
Research areas and keywords

Subject classification (UKÄ) – MANDATORY

  • Radiology, Nuclear Medicine and Medical Imaging
Original languageEnglish
Pages (from-to)265-268
JournalJournal of Radioanalytical and Nuclear Chemistry
Volume277
Issue number1
Publication statusPublished - 2008
Publication categoryResearch
Peer-reviewedYes