A Continuum Theory of Phase Separation Kinetics for Active Brownian Particles

Joakim Stenhammar, Adriano Tiribocchi, Rosalind J. Allen, Davide Marenduzzo, Michael E. Cates

Forskningsoutput: TidskriftsbidragLetterPeer review

340 Nedladdningar (Pure)

Sammanfattning

Active Brownian particles (ABPs), when subject to purely repulsive interactions, are known to undergo activity-induced phase separation broadly resembling an equilibrium (attraction-induced) gas-liquid coexistence. Here we present an accurate continuum theory for the dynamics of phase-separating ABPs, derived by direct coarse-graining, capturing leading-order density gradient terms alongside an effective bulk free energy. Such gradient terms do not obey detailed balance; yet we find coarsening dynamics closely resembling that of equilibrium phase separation. Our continuum theory is numerically compared to large-scale direct simulations of ABPs and accurately accounts for domain growth kinetics, domain topologies and coexistence densities.
Originalspråkengelska
Artikelnummer145702
TidskriftPhysical Review Letters
Volym111
DOI
StatusPublished - 2013

Ämnesklassifikation (UKÄ)

  • Fysikalisk kemi (Här ingår: Yt- och kolloidkemi)

Fingeravtryck

Utforska forskningsämnen för ”A Continuum Theory of Phase Separation Kinetics for Active Brownian Particles”. Tillsammans bildar de ett unikt fingeravtryck.

Citera det här