Deep Inner-Shell Multiphoton Ionization by Intense X-Ray Free-Electron Laser Pulses

H. Fukuzawa; S. -K. Son; K. Motomura; S. Mondal; K. Nagaya; S. Wada; X. -J. Liu; R. Feifel; T. Tachibana; Y. Ito; M. Kimura; T. Sakai; K. Matsunami; H. Hayashita; J. Kajikawa; Per Johnsson; M. Siano; E. Kukk; B. Rudek; B. Erk; L. Foucar; E. Robert; C. Miron; K. Tono; Y. Inubushi; T. Hatsui; M. Yabashi; M. Yao; R. Santra; K. Ueda

doi:10.1103/PhysRevLett.110.173005

Deep Inner-Shell Multiphoton Ionization by Intense X-Ray Free-Electron Laser Pulses

H. Fukuzawa, S. -K. Son, K. Motomura, S. Mondal, K. Nagaya, S. Wada, X. -J. Liu, R. Feifel, T. Tachibana, Y. Ito, M. Kimura, T. Sakai, K. Matsunami, H. Hayashita, J. Kajikawa, Per Johnsson, M. Siano, E. Kukk, B. Rudek, B. ErkL. Foucar, E. Robert, C. Miron, K. Tono, Y. Inubushi, T. Hatsui, M. Yabashi, M. Yao, R. Santra, K. Ueda

Atomfysik

Forskningsoutput: Tidskriftsbidrag › Artikel i vetenskaplig tidskrift › Peer review

Sammanfattning

We have investigated multiphoton multiple ionization dynamics of xenon atoms using a new x-ray free-electron laser facility, SPring-8 Angstrom Compact free electron LAser (SACLA) in Japan, and identified that Xen+ with n up to 26 is produced at a photon energy of 5.5 keV. The observed high charge states (n >= 24) are produced via five-photon absorption, evidencing the occurrence of multiphoton absorption involving deep inner shells. A newly developed theoretical model, which shows good agreement with the experiment, elucidates the complex pathways of sequential electronic decay cascades accessible in heavy atoms. The present study of heavy-atom ionization dynamics in high-intensity hard-x-ray pulses makes a step forward towards molecular structure determination with x-ray free-electron lasers. DOI: 10.1103/PhysRevLett.110.173005

Originalspråk	engelska
Artikelnummer	173005
Tidskrift	Physical Review Letters
Volym	110
Nummer	17
DOI	https://doi.org/10.1103/PhysRevLett.110.173005
Status	Published - 2013

Ämnesklassifikation (UKÄ)

Atom- och molekylfysik och optik

Tillgång till dokument

10.1103/PhysRevLett.110.173005

Citera det här

Fukuzawa, H., Son, S. .-K., Motomura, K., Mondal, S., Nagaya, K., Wada, S., Liu, X. .-J., Feifel, R., Tachibana, T., Ito, Y., Kimura, M., Sakai, T., Matsunami, K., Hayashita, H., Kajikawa, J., Johnsson, P., Siano, M., Kukk, E., Rudek, B., ... Ueda, K. (2013). Deep Inner-Shell Multiphoton Ionization by Intense X-Ray Free-Electron Laser Pulses. Physical Review Letters, 110(17), Artikel 173005. https://doi.org/10.1103/PhysRevLett.110.173005

@article{90709c200f814fa3a21bc1a8f3e75bdb,

title = "Deep Inner-Shell Multiphoton Ionization by Intense X-Ray Free-Electron Laser Pulses",

abstract = "We have investigated multiphoton multiple ionization dynamics of xenon atoms using a new x-ray free-electron laser facility, SPring-8 Angstrom Compact free electron LAser (SACLA) in Japan, and identified that Xen+ with n up to 26 is produced at a photon energy of 5.5 keV. The observed high charge states (n >= 24) are produced via five-photon absorption, evidencing the occurrence of multiphoton absorption involving deep inner shells. A newly developed theoretical model, which shows good agreement with the experiment, elucidates the complex pathways of sequential electronic decay cascades accessible in heavy atoms. The present study of heavy-atom ionization dynamics in high-intensity hard-x-ray pulses makes a step forward towards molecular structure determination with x-ray free-electron lasers. DOI: 10.1103/PhysRevLett.110.173005",

author = "H. Fukuzawa and Son, {S. -K.} and K. Motomura and S. Mondal and K. Nagaya and S. Wada and Liu, {X. -J.} and R. Feifel and T. Tachibana and Y. Ito and M. Kimura and T. Sakai and K. Matsunami and H. Hayashita and J. Kajikawa and Per Johnsson and M. Siano and E. Kukk and B. Rudek and B. Erk and L. Foucar and E. Robert and C. Miron and K. Tono and Y. Inubushi and T. Hatsui and M. Yabashi and M. Yao and R. Santra and K. Ueda",

year = "2013",

doi = "10.1103/PhysRevLett.110.173005",

language = "English",

volume = "110",

journal = "Physical Review Letters",

issn = "1079-7114",

publisher = "American Physical Society",

number = "17",

}

Fukuzawa, H, Son, S-K, Motomura, K, Mondal, S, Nagaya, K, Wada, S, Liu, X-J, Feifel, R, Tachibana, T, Ito, Y, Kimura, M, Sakai, T, Matsunami, K, Hayashita, H, Kajikawa, J, Johnsson, P, Siano, M, Kukk, E, Rudek, B, Erk, B, Foucar, L, Robert, E, Miron, C, Tono, K, Inubushi, Y, Hatsui, T, Yabashi, M, Yao, M, Santra, R & Ueda, K 2013, 'Deep Inner-Shell Multiphoton Ionization by Intense X-Ray Free-Electron Laser Pulses', Physical Review Letters, vol. 110, nr. 17, 173005. https://doi.org/10.1103/PhysRevLett.110.173005

TY - JOUR

T1 - Deep Inner-Shell Multiphoton Ionization by Intense X-Ray Free-Electron Laser Pulses

AU - Fukuzawa, H.

AU - Son, S. -K.

AU - Motomura, K.

AU - Mondal, S.

AU - Nagaya, K.

AU - Wada, S.

AU - Liu, X. -J.

AU - Feifel, R.

AU - Tachibana, T.

AU - Ito, Y.

AU - Kimura, M.

AU - Sakai, T.

AU - Matsunami, K.

AU - Hayashita, H.

AU - Kajikawa, J.

AU - Johnsson, Per

AU - Siano, M.

AU - Kukk, E.

AU - Rudek, B.

AU - Erk, B.

AU - Foucar, L.

AU - Robert, E.

AU - Miron, C.

AU - Tono, K.

AU - Inubushi, Y.

AU - Hatsui, T.

AU - Yabashi, M.

AU - Yao, M.

AU - Santra, R.

AU - Ueda, K.

PY - 2013

Y1 - 2013

N2 - We have investigated multiphoton multiple ionization dynamics of xenon atoms using a new x-ray free-electron laser facility, SPring-8 Angstrom Compact free electron LAser (SACLA) in Japan, and identified that Xen+ with n up to 26 is produced at a photon energy of 5.5 keV. The observed high charge states (n >= 24) are produced via five-photon absorption, evidencing the occurrence of multiphoton absorption involving deep inner shells. A newly developed theoretical model, which shows good agreement with the experiment, elucidates the complex pathways of sequential electronic decay cascades accessible in heavy atoms. The present study of heavy-atom ionization dynamics in high-intensity hard-x-ray pulses makes a step forward towards molecular structure determination with x-ray free-electron lasers. DOI: 10.1103/PhysRevLett.110.173005

AB - We have investigated multiphoton multiple ionization dynamics of xenon atoms using a new x-ray free-electron laser facility, SPring-8 Angstrom Compact free electron LAser (SACLA) in Japan, and identified that Xen+ with n up to 26 is produced at a photon energy of 5.5 keV. The observed high charge states (n >= 24) are produced via five-photon absorption, evidencing the occurrence of multiphoton absorption involving deep inner shells. A newly developed theoretical model, which shows good agreement with the experiment, elucidates the complex pathways of sequential electronic decay cascades accessible in heavy atoms. The present study of heavy-atom ionization dynamics in high-intensity hard-x-ray pulses makes a step forward towards molecular structure determination with x-ray free-electron lasers. DOI: 10.1103/PhysRevLett.110.173005

U2 - 10.1103/PhysRevLett.110.173005

DO - 10.1103/PhysRevLett.110.173005

M3 - Article

C2 - 23679721

SN - 1079-7114

VL - 110

JO - Physical Review Letters

JF - Physical Review Letters

IS - 17

M1 - 173005

ER -

Deep Inner-Shell Multiphoton Ionization by Intense X-Ray Free-Electron Laser Pulses

Sammanfattning

Ämnesklassifikation (UKÄ)

Tillgång till dokument

Fingeravtryck

Citera det här