Free-Standing Metal Halide Perovskite Nanowire Arrays with Blue-Green Heterostructures

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Sammanfattning

Vertically aligned metal halide perovskite (MHP) nanowires are promising for various optoelectronic applications, which can be further enhanced by heterostructures. However, present methods to obtain free-standing vertically aligned MHP nanowire arrays and heterostructures lack the scalability needed for applications. We use a low-temperature solution process to prepare free-standing vertically aligned green-emitting CsPbBr3 nanowires from anodized aluminum oxide templates. The length is controlled from 1 to 20 μm by the precursor amount. The nanowires are single-crystalline and exhibit excellent photoluminescence, clear light guiding and high photoconductivity with a responsivity of 1.9 A/W. We demonstrate blue-green heterostructured nanowire arrays by converting the free-standing part of the nanowires to CsPbCl1.1Br1.9 in an anion exchange process. Our results demonstrate a scalable, self-aligned, and lithography-free approach to achieve high quality free-standing MHP nanowires arrays and heterostructures, offering new possibilities for optoelectronic applications.

Originalspråkengelska
Sidor (från-till)2941-2947
TidskriftNano Letters
Volym22
Nummer7
DOI
StatusPublished - 2022

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© 2022 The Authors. Published by American Chemical Society.

Ämnesklassifikation (UKÄ)

  • Den kondenserade materiens fysik

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